a dense, dark cloud, especially a heavy storm or rain cloud
This is the Bible's word for the thick, dark cloud, the heavy mass of cloud that piles up in the sky and lets down rain. It is a more specific word than the ordinary term for a cloud: where that general word can name any cloud (including the bright pillar that led Israel), this one leans toward the dark, water-laden storm cloud, the kind that gathers, thickens, and bursts.
Because of that, its natural home is weather. Clouds here rise from the sea before a downpour, blacken the sky, are loaded with moisture, pour out water, and are ordered to withhold rain in judgment. Even where the word is used for a picture (favor that comes like a rain cloud, sins that are wiped away like a cloud, a life that passes as swiftly as a cloud), the image behind it is still this heavy cloud of the sky.
The same dark storm cloud is also how the poets saw God arrive. When the Lord comes down in power he comes veiled in thick cloud, makes the clouds his chariot, and rides on a swift cloud. So the one word covers both the ordinary weather overhead and the storm in which God shows his presence and majesty.